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Modeling and diagnosis of the stratospheric circulation / Edward Joseph Charlesworth. Wuppertal, December 14, 2021
Content
Introduction
Background
Radiation
Stratospheric Transport
Early Theory Development
The Residual Circulation
A Comprehensive Circulation
Stratospheric Polar Vortices
Chemicals and Tracers
Water Vapor
Ozone
Chapman Chemistry
Other Destruction
Effect of Transport
Other Chemicals
Age of Air
Expected Trends
Temperature
Water Vapor
Ozone
Residual Circulation
The Development of Stratospheric Transport Models
Modeling Stratospheric Transport
Introduction
EMAC-CLaMS and EMAC-FFSL
Models
Calculation of Age Spectra in a Model
Forward Tracers
The EMAC-CLaMS Lower and Upper Boundary
Differences in the Zonal Mean State: Global Perspective
Mean age of air
Chemical Composition
Inter-annual variability
Age spectrum shape
Differences in the representation of transport processes
Tropical and mid-latitude stratosphere
Lowermost Stratosphere
Discussion
Conclusions
Radiative Effects of Stratospheric Water Vapor
Radiative Coupling
Experiment Design
Water Differences
Water Vapor Distribution Differences in Uncoupled Simulation
Temperature Differences
Recent Literature Context
Conclusions
Quantifying Brewer-Dobson Circulation Variability from Ozone Observations
Current Knowledge
Effective Upwelling
Validity of Proxy Assumption
Upwelling Seasonal Cycle
Timeseries
Correlations with Reanalyses
Limitations of the Method
Validity at other levels
Application of SHADOZ data
Calculation of Photolysis Rates
Simple Calculation
Discussion
Conclusions
A Closing Word
Bibliography
Photolysis of Diatomic Oxygen