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Carbonyl sulfide in the stratosphere : airborne instrument development and satellite based data analysis / Corinna Kloss. Jülich : Forschungszentrum Jülich GmbH, Zentralbibliothek, [2017] ; © 2017
Inhalt
Introduction
The upper troposphere and stratosphere
Stratospheric aerosol and OCS
Transport of sulfur compounds into the stratosphere
Role, mixing ratio and budget of Carbonyl Sulfide
OCS trends and seasonality
OCS observations
Remote sensing
In-situ observations
Motivation for the Airborne Mid-Infrared Cavity enhanced Absorption spectrometer (AMICA)
M55 Geophysica observations during StratoClim
Stratospheric OCS with ACE-FTS
ACE-FTS OCS data product
ACE-FTS satellite sampling bias correction
Motivation
Bodeker Scientific Regression Model (BSRM)
The BSRM performance with the OCS ACE-FTS data set
Sampling bias correction procedure
Evaluation of the correction procedure
Comparison with MIPAS
OCS burden
Seasonal and zonal variations
Tropopause effects
Stratospheric global OCS burden
Asian monsoon
AMICA development
Infrared spectroscopy
The ICOS method
Requirements for OCS measurements
MICA
Material criteria
Calibration system for OCS
OCS calibration and comparison with Mainz LGR
Mechanical requirements for AMICA on the research aircraft Geophysica
Mechanical design of AMICA
Laboratory performance assessment
Flow system assessment
Test enclosure
Flight simulation experiment with AMICA
AMICA performance
Performance of AMICA during first measurement flights
OCS calibration
AMICA results
Measurements
OCS and CO in the UTLS and stratosphere
Asian monsoon influence
A first AMICA and ACE-FTS comparison
Conclusions and outlook
Bibliography
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