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Stratospheric ClOOCl chemistry at high solar zenith angles / von Olga Suminska-Ebersoldt. 2012
Content
Ozone in the stratosphere
Natural stratosphere
Stratospheric ozone chemistry
Dynamics of the stratosphere
Anthropogenic perturbations to stratospheric ozone
Chlorine in the stratosphere
Heterogeneous chemistry
Stratospheric ClO/ClOOCl chemistry
Antarctic: Ozone hole
Arctic: Ozone loss
The ClO dimer cycle
Recombination and dissociation constants
Equilibrium constant
Photolysis rate
Photolysis quantum yield
Absorption/photolysis cross sections
Actinic flux
The HALOX instrument
The CCRF technique in ClO detection
Calibration
The instrument configuration
Chemistry transport and radiative transfer models
The CLaMS Model
Radiative transfer models
libRadtran software package
UMD radiative transfer model
The self-match flight
Measurements
Matches
Equilibrium constant estimation
Backward trajectories analysis
Night-time ClOx chemistry
Actinic flux in the lower stratosphere
Model comparison for clear sky conditions
Sensitivity studies
Ozone
Albedo
Clouds
Aerosol
Refraction
Constraints on the ClOOCl photolysis rate
Investigated ClOOCl cross sections/spectra
Constraints on ClOOCl photolysis from the observed increase in ClO
Chemistry simulations along match trajectories
Summary and outlook
Conclusions
Outlook
References