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Structural and optoelectronic properties, phase transitions, and degradation of semiconducting CsPbI3-perovskite thin films for photovoltaics / by Pascal Becker ; Helmholtz Zentrum Berlin, Bergische Universität Wuppertal. Wuppertal, 2019
Content
1 Introduction
2 Material Background, Sample Preparation and Characterization Techniques
2.1 Fully Inorganic CsPbI3-Perovskite
2.2 Characterization Techniques
2.3 Evaporation Chamber with In-Situ Characterization
2.4 CsPbI3 Thin-Film Preparation and Application
3 Growth and Physical Properties of Co-Evaporated CsPbI3 Thin-Films
3.1 Sample Preparation Procedure and Appearance
3.2 Elemental Composition
3.3 Crystal Structure
3.4 Surface Morphology
3.5 In-Situ Monitoring of Optical Properties During the Deposition
4 Optoelectronic Properties of As-Deposited Films
4.1 Optical Properties
4.2 Charge Carrier Generation and Recombination
4.3 Charge Carrier Dynamics
4.4 Application in Photovoltaic Devices - Solar Cell Performance
5 High Temperature Phase Transition
5.1 Annealing Procedure
5.2 In-Situ Monitoring of the Optical Reflection
5.3 Elemental Composition
5.4 Crystal Structure
5.5 Surface Morphology
5.6 Optoelectronic Properties
6 Degradation Causes and Principle
6.1 In-Situ Monitoring of the Crystal Structure During Degradation
6.2 In-Situ Reflection Imaging during Degradation
6.3 Causes and Model of the Degradation Process
6.4 Optical Properties after Degradation
7 Conclusions
8 Outlook
9 References
A Appendix
B Appendix